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    Method for surface modification of molded article of plastic and method for modifying polymer
    1.
    发明授权
    Method for surface modification of molded article of plastic and method for modifying polymer 失效
    塑料模塑制品的表面改性方法和改性聚合物的方法

    公开(公告)号：US06486265B1

    公开(公告)日：2002-11-26

    申请号：US09719395

    申请日：2001-02-22

    申请人： Yasutaka Ishii ,  Yoshinori Funaki ,  Tatsuya Nakano

    发明人： Yasutaka Ishii ,  Yoshinori Funaki ,  Tatsuya Nakano

    IPC分类号： C08F800

    CPC分类号： C08J7/12

    摘要： An invented method for the surface modification of a molded plastic treats a molded plastic with an oxygen-atom-containing gas such as oxygen, carbon monoxide, a nitrogen oxide, or a sulfur oxide in the presence of N-hydroxyphthalimide or another imide compound represented by the following formula (1): wherein R1 and R2 are each, identical to or different from each other, a hydrogen atom, a halogen atom, an alkyl group, an aryl group, a cycloalkyl group, a hydroxyl group, an alkoxy group, a carboxyl group, an alkoxycarbonyl group, or an acyl group, or R1 and R2 may be combined to form a double bond or an aromatic or non-aromatic ring; X is an oxygen atom or a hydroxyl group. An invented method for modifying a polymer treats a polymer with an oxygen-atom-containing gas such as oxygen, carbon monoxide, a nitrogen oxide, or a sulfur oxide in the presence of the imide compound represented by the formula (1).

    摘要翻译： 用于模塑塑料的表面改性的发明方法在N-羟基邻苯二甲酰亚胺或其它酰亚胺化合物的存在下，用含氧原子的气体例如氧，一氧化碳，氮氧化物或硫氧化物处理模塑塑料 通过下式（1）表示：其中R 1和R 2各自彼此相同或不同，为氢原子，卤素原子，烷基，芳基，环烷基，羟基，烷氧基 ，羧基，烷氧基羰基或酰基，或者R 1和R 2可以结合形成双键或芳族或非芳族环; X是氧原子或羟基。 在式（1）表示的酰亚胺化合物的存在下，本发明的改性聚合物可以用含氧原子的气体如氧，一氧化碳，氮氧化物或硫氧化物处理聚合物。

    Process for the preparation of furan compounds
    3.
    发明申请
    Process for the preparation of furan compounds 失效
    呋喃化合物的制备方法

    公开(公告)号：US20070197806A1

    公开(公告)日：2007-08-23

    申请号：US11709203

    申请日：2007-02-22

    申请人： Yasutaka Ishii ,  Tatsuya Nakano ,  Takahiro Iwahama

    发明人： Yasutaka Ishii ,  Tatsuya Nakano ,  Takahiro Iwahama

    IPC分类号： C07D307/02

    CPC分类号： C07D307/68 ,  C07D307/46

    摘要： A carbonyl compound represented by following Formula (1): wherein R1 represents hydrogen atom or an organic group; and R2 represents hydrogen atom or an organic group having a carbon atom at a bonding site with the carbonyl group in Formula (1), wherein R1 and R2 may be combined to form a ring with adjacent two carbon atoms, or an equivalent thereof is reacted with an unsaturated compound represented by following Formula (2): wherein each of R3, R4, and R5 represents hydrogen atom, a halogen atom, hydroxyl group, or an organic group and wherein R3 and R4 may be combined to form a ring with adjacent two carbon atoms, or a precursor thereof, to yield a furan compound represented by following Formula (3): wherein R3′ represents R3, R5 or hydrogen atom; and R1, R2, R3, R4, are R5 are as defined above.

    摘要翻译： 由下式（1）表示的羰基化合物：其中R 1表示氢原子或有机基团; R 2表示氢原子或在式（1）中与羰基键合位置具有碳原子的有机基团，其中R 1和R 2各自独立地表示氢原子， 2可以组合形成具有相邻两个碳原子的环，或者其等同物与下式（2）表示的不饱和化合物反应：其中R 3，R 3， R 4和R 5代表氢原子，卤素原子，羟基或有机基团，并且其中R 3和R 3各自独立地选自氢， 4可以组合形成具有相邻的两个碳原子的环或其前体，得到由下式（3）表示的呋喃化合物：其中R 3表示R' SO 3，R 5或氢原子; R 1，R 2，R 3，R 4，R 4，R 5，R 4， >如上所定义。

    Process for producing vinyl ether compounds
    4.
    发明授权
    Process for producing vinyl ether compounds 失效
    制备乙烯基醚化合物的方法

    公开(公告)号：US07074970B2

    公开(公告)日：2006-07-11

    申请号：US10231115

    申请日：2002-08-30

    申请人： Yasutaka Ishii ,  Tatsuya Nakano ,  Keizo Inoue

    发明人： Yasutaka Ishii ,  Tatsuya Nakano ,  Keizo Inoue

    IPC分类号： C07C43/00

    CPC分类号： C07D313/10 ,  C07C41/16 ,  C07C43/162 ,  C07C49/753 ,  C07C69/757 ,  C07C2601/14 ,  C07C2603/74 ,  C07C2603/86 ,  C07D307/33 ,  C07D307/93 ,  Y02P20/55 ,  C07C43/16 ,  C07C43/168 ,  C07C43/178 ,  C07C43/188 ,  C07C43/215

    摘要： A process produces vinyl ether compounds and includes allowing a vinyl ester compound represented by following Formula (1): wherein R1, R2, R3 and R4 are the same or different and are each a hydrogen atom or an organic group, to react with a hydroxy compound represented by following Formula (2): R5OH  (2) wherein R5 is an organic group, in the presence of at least one transition element compound to thereby yield a vinyl ether compound represented by following Formula (3): wherein R2, R3, R4 and R5 have the same meanings as defined above. Such transition element compounds include iridium compounds and other compounds containing Group VIII elements.

    摘要翻译： 一种方法制备乙烯基醚化合物，包括使下式（1）表示的乙烯基酯化合物：其中R 1，R 2，R 3， >和R 4相同或不同，并且各自为氢原子或有机基团，与下式（2）表示的羟基化合物反应：<？在线式描述= “在线公式”end =“lead”？> 5 OH（2）<？in-line-formula description =“In-line Formulas”end =“tail”？>其中R 在至少一种过渡元素化合物的存在下，有机基团是有机基团，从而得到下式（3）表示的乙烯基醚化合物：其中R 2，R R 4，R 4和R 5具有与上述相同的含义。 这种过渡元素化合物包括铱化合物和含有VIII族元素的其它化合物。

    Oxygenation catalyst and process for producing a ketone using the same
    5.
    发明授权
    Oxygenation catalyst and process for producing a ketone using the same 失效
    氧合催化剂及其制备方法

    公开(公告)号：US06232258B1

    公开(公告)日：2001-05-15

    申请号：US09072354

    申请日：1998-05-05

    申请人： Yasutaka Ishii ,  Tatsuya Nakano

    发明人： Yasutaka Ishii ,  Tatsuya Nakano

    IPC分类号： B01J3102

    CPC分类号： B01J31/34 ,  B01J31/006 ,  B01J31/0247 ,  B01J31/2208 ,  B01J31/36 ,  B01J2231/70 ,  B01J2531/56 ,  C07C29/50 ,  C07C45/33 ,  C07C45/34 ,  C07C45/36 ,  C07C49/453 ,  C07C2603/74 ,  C07C35/37

    摘要： A substrate is contacted with oxygen in the presence of the imide compound shown by the following formula (1) (N-hydroxyphthalimide) and a strong acid, or the imide compound, the strong acid and a co-catalyst (e.g., a transition metal compound) to oxygenate the substrate with high conversion and selectivity: wherein R1 and R2 represent a substituent such as a hydrogen atom or a halogen atom, an alkyl group, an aryl group or a cycloalkyl group, or R1 and R2 may bond together to form a double bond or an aromatic or nonaromatic ring, X is O or OH, and n is 1 to 3. The substrate comprises, for example, at least one compound selected from (a) a compound having a methyl group or a methylene group at an adjacent site of an unsaturated bond, (b) a homo- or hetero cyclic compound having a methylene group, (c) a compound having a methine carbon atom, (d) a compound having a methyl group or a methylene group at an adjacent site of an aromatic ring and (e) a compound having a methyl group or a methylene group at an adjacent site of a carbonyl group.

    摘要翻译： 存在下式（1）所示的酰亚胺化合物（N-羟基邻苯二甲酰亚胺）和强酸或酰亚胺化合物，强酸和助催化剂（例如过渡金属 化合物）以高转化率和选择性对底物进行含氧化：其中R1和R2表示取代基如氢原子或卤素原子，烷基，芳基或环烷基，或R1和R2可以键合在一起形成 双键或芳族或非芳族环，X为O或OH，n为1至3.底物包含例如至少一种选自（a）具有甲基或亚甲基的化合物的化合物， 不饱和键的相邻位置，（b）具有亚甲基的均聚或杂环化合物，（c）具有次甲基碳原子的化合物，（d）相邻的具有甲基或亚甲基的化合物 芳环的位置和（e）具有甲基或甲基的化合物 烯基在羰基的相邻位置。

    Oxidation process of branched aliphatic hydrocarbons and process for producing the oxide
    7.
    发明授权
    Oxidation process of branched aliphatic hydrocarbons and process for producing the oxide 失效
    支链脂族烃的氧化过程及其制备方法

    公开(公告)号：US6037507A

    公开(公告)日：2000-03-14

    申请号：US37703

    申请日：1998-03-10

    申请人： Tatsuya Nakano ,  Yasutaka Ishii

    发明人： Tatsuya Nakano ,  Yasutaka Ishii

    IPC分类号： B01J31/02 ,  B01J31/04 ,  C07B41/02 ,  C07B41/06 ,  C07B61/00 ,  C07C27/12 ,  C07C29/50 ,  C07C31/12 ,  C07C45/28 ,  C07C45/33 ,  C07C49/08 ,  C07C31/04

    CPC分类号： C07C45/33 ,  C07C29/50

    摘要： A non-cyclic branched aliphatic hydrocarbon (e.g., isobutane) is oxidized with oxygen in the presence of an oxidation catalyst comprising an imide compound of the following formula (1) (e.g., N-hydroxyphthalimide) or an oxidation catalyst comprising the imide compound and a co-catalyst (e.g., a transition metal compound of selected from Group 3A, 4A, 5A, 6A, 7A, 8 and 1B elements of the Periodic Table of elements), for the formation of an oxide (e.g., t-butanol, acetone): ##STR1## wherein R.sup.1 and R.sup.2 represent a substituent such as a hydrogen atom or a halogen atom, or R.sup.1 and R.sup.2 may together form a double bond or an aromatic or non-aromatic 5- to 12-membered ring, X is O or OH, and n is 1 to 3.

    摘要翻译： 在包含下式（1）的酰亚胺化合物的氧化催化剂（例如，N-羟基邻苯二甲酰亚胺）或包含酰亚胺化合物的氧化催化剂的存在下，用氧氧化非环状支链脂族烃（例如异丁烷） 助催化剂（例如，选自元素周期表的3A，4A，5A，6A，7A，8和1B族元素的过渡金属化合物），用于形成氧化物（例如，叔丁醇， 丙酮）：其中R 1和R 2表示取代基如氢原子或卤素原子，或者R 1和R 2可以一起形成双键或芳族或非芳族的5至12元环，X是O或OH ，n为1〜3。

    Method for producing nitro compounds
    9.
    发明授权
    Method for producing nitro compounds 失效
    硝基化合物的制备方法

    公开(公告)号：US5956657A

    公开(公告)日：1999-09-21

    申请号：US997585

    申请日：1997-12-23

    申请人： Tatsuya Nakano ,  Satoshi Sakaguchi ,  Yasutaka Ishii

    发明人： Tatsuya Nakano ,  Satoshi Sakaguchi ,  Yasutaka Ishii

    IPC分类号： C07B43/02 ,  C07C201/08 ,  C07C205/04 ,  C07C205/05 ,  C07C205/00

    CPC分类号： C07B43/02 ,  C07C201/08 ,  C07C2103/74

    摘要： The method provides nitro compounds at a high conversion and selectivity by nitrating substrates under comparatively mild conditions in the absence of catalysts. Organic substrates are nitrated using no catalysts or ozone, but using (1) at least one nitrogen compound selected from N.sub.2 O or NO and oxygen. It is advantageous for the nitration reaction to employ a nitrogen compound obtained by a reaction of the nitrogen compound with oxygen, particularly a nitrogen oxide comprising N.sub.2 O.sub.3 as a main component. Additionally, organic substrates are nitrated using (2) NO.sub.2. The substrates include a compound having a methine-carbon atom, and a compound having a methyl group or methylene group in an adjacent position to an aromatic ring.

    摘要翻译： 该方法通过在不存在催化剂的情况下在相对温和的条件下硝化底物以高转化率和选择性提供硝基化合物。 使用没有催化剂或臭氧的有机底物进行硝化，但使用（1）至少一种选自N 2 O或NO的氮化合物和氧气。 硝化反应采用氮化合物与氧反应获得的氮化合物，特别是以N 2 O 3为主要成分的氮氧化物是有利的。 另外，使用（2）NO2对有机底物进行硝化。 底物包括具有次甲基 - 碳原子的化合物和在芳香环相邻位置具有甲基或亚甲基的化合物。