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    Catalyst, its preparation and its use in a dehydrogenation process
    1.
    发明申请
    Catalyst, its preparation and its use in a dehydrogenation process 有权
    催化剂，其制备及其在脱氢方法中的应用

    公开(公告)号：US20030144566A1

    公开(公告)日：2003-07-31

    申请号：US10352819

    申请日：2003-01-28

    Inventor： Robert Dielman Culp ,  Eugene Harry Theobald ,  Sarah Louise Weaver

    IPC: C07C005/32 ,  C07C005/333

    CPC classification number: C07C5/3332 ,  B01J23/83 ,  B01J23/85 ,  B01J23/8871 ,  B01J37/088 ,  C07C2523/04 ,  C07C2523/10 ,  C07C2523/28 ,  C07C2523/745 ,  C07C15/44 ,  C07C15/46

    Abstract: A catalyst which is based upon an iron oxide and a compound of a lanthanide, of which iron oxide at least a portion is made by a process which involves heat decomposition of an iron halide, the lanthanide being in a quantity in the range of from 0.07 to 0.15 mole per mole iron oxide present in the catalyst, calculated as Fe2O3; a process for the preparation of the catalyst; a process for the dehydrogenation of an alkylaromatic compound which process involves contacting a feed containing the alkylaromatic compound with the catalyst; and a method of using an alkenylaromatic compound for making polymers or copolymers, in which method the alkenylaromatic compound has been prepared by the dehydrogenation process.

    Abstract translation: 一种催化剂，其基于氧化铁和镧系化合物，其中氧化铁至少一部分通过涉及卤化铁的热分解的方法制备，所述镧系元素的量为0.07 至0.15摩尔/摩尔氧化铁存在于催化剂中，以Fe 2 O 3计算; 催化剂的制备方法; 烷基芳族化合物脱氢的方法，该方法包括使含有烷基芳族化合物的进料与催化剂接触; 以及使用链烯基芳族化合物制造聚合物或共聚物的方法，其中通过脱氢方法制备了链烯基芳族化合物。

    Process for the production of olefins
    2.
    发明申请
    Process for the production of olefins 审中-公开
    烯烃生产工艺

    公开(公告)号：US20030055306A1

    公开(公告)日：2003-03-20

    申请号：US10168482

    申请日：2002-09-04

    Inventor： John Wiliiam Couves ,  David Charles Griffiths ,  Brian Edward Messenger

    IPC: C07C005/373 ,  C07C005/333

    CPC classification number: C07C5/48 ,  C07C2523/62 ,  Y02P20/52 ,  C07C11/02 ,  C07C11/04

    Abstract: A process for the production of an olefin from a hydrocarbon, which process comprises: partially combusting the hydrocarbon and an oxygen-containing gas in the presence of a catalyst, characterised in that the catalyst comprises platinum and at least one further metal, said further metal being a Group IIIA, Group IVA, VA or a transition metal; wherein said catalyst is: a) not a platinum catalyst consisting essentially of platinum modified with Sn, Cu or mixtures thereof, and b) not a platinum catalyst consisting essentially of platinum modified with Sb or a mixture of Sb and Sn.

    Abstract translation: 一种从烃生产烯烃的方法，该方法包括：在催化剂存在下部分地燃烧烃和含氧气体，其特征在于催化剂包含铂和至少一种其它金属，所述另外的金属 作为IIIA族，IVA族，VA族或过渡金属; 其中所述催化剂是：a）不是基本上由Sn，Cu或其混合物改性的铂组成的铂催化剂，和b）不是主要由Sb改性的铂或Sb和Sn的混合物组成的铂催化剂。

    Process for preparing light olefins by dehydrogenation of the corresponding paraffins
    3.
    发明申请
    Process for preparing light olefins by dehydrogenation of the corresponding paraffins 失效
    通过相应的链烷烃的脱氢制备轻质烯烃的方法

    公开(公告)号：US20020198428A1

    公开(公告)日：2002-12-26

    申请号：US10184888

    申请日：2002-07-01

    Applicant: SNAMPROGETTI S.p.A.

    Inventor： Rodolfo Iezzi ,  Andrea Bartolini ,  Franco Buonomo

    IPC: C07C005/327 ,  C07C005/32 ,  C07C005/333

    CPC classification number: B01J23/96 ,  B01J8/0055 ,  B01J8/26 ,  B01J23/62 ,  C07C5/3337 ,  Y02P20/584 ,  C07C11/02

    Abstract: A process for preparing light olefins from corresponding paraffins consists of reacting said paraffins in a reactor, operating at a temperature of between 450 and 800null C., a pressure of between 0.1 and 3 atm absolute and a GHSV of between 100 and 10000 hnull1, with a catalytic system containing gallium, platinum, possibly one or more alkaline or alkaline-earth metals, and a support consisting of alumina in delta or theta phase or in deltanulltheta or thetanullalpha or deltanullthetanullalpha mixed phase, modified with silica, the gallium, expressed as Ga2O3, being in a quantity of between 0.1 and 33.6 wt %, the platinum being in a quantity of between 1 and 99 ppm, the alkaline or alkaline-earth metals, expressed as oxide, being in a quantity of between 0 and 5 wt %, and the silica being in a quantity of between 0.08 and 3 wt %, the rest to 100% being alumina, and regenerating said catalytic system in a regenerator by burning off the coke which has deposited on its surface, without subsequently reducing it.

    Abstract translation: 从相应的链烷烃制备轻质烯烃的方法包括在反应器中使所述链烷烃反应，在450-800℃的温度下操作，绝对压力为0.1至3atm，GHSV为100至10000h- 1，含有镓，铂，可能一种或多种碱金属或碱土金属的催化体系，以及由δ或θ相中的氧化铝或δ+θ或θ+α或δ+θ+α混合相组成的载体 ，用二氧化硅改性，以Ga 2 O 3表示的镓的量为0.1至33.6重量％，铂的量为1至99ppm，碱或碱土金属以氧化物表示，为 其量为0至5重量％，二氧化硅的量为0.08至3重量％，其余为100重量％的氧化铝，并通过烧掉已沉积的焦炭在再生器中再生所述催化体系 在其表面，没有随后减少 把它。

    Zeolite-based catalyst material, the preparation thereof and the use thereof for the selective dehydrogenation of n-butane
    4.
    发明申请
    Zeolite-based catalyst material, the preparation thereof and the use thereof for the selective dehydrogenation of n-butane 审中-公开
    沸石催化剂材料，其制备方法及其用于正丁烷选择性脱氢的用途

    公开(公告)号：US20020161271A1

    公开(公告)日：2002-10-31

    申请号：US10136904

    申请日：2002-05-02

    Applicant: Phillips Petroleum Company

    Inventor： An-hsiang Wu ,  Charles A. Drake

    IPC: C07C005/333 ,  B01J029/62

    CPC classification number: B01J29/605 ,  B01J29/60 ,  B01J37/0009

    Abstract: A process in which a hydrocarbon feedstock containing n-butane is selectively dehydrogenated to a product containing butenes. A catalyst suitable for the selective dehydrogenation of a feedstock containing n-butane to provide a product containing butenes. A method for producing a catalyst suitable for the selective dehydrogenation of a feedstock containing n-butane to provide a product containing butenes.

    Abstract translation: 将含有正丁烷的烃原料选择性脱氢成含有丁烯的产物的方法。 适用于含有正丁烷的原料的选择性脱氢以提供含有丁烯的产物的催化剂。 一种用于制备适于含有正丁烷的原料的选择性脱氢以提供含有丁烯的产物的催化剂的方法。

    Dehydrogenation process
    5.
    发明申请
    Dehydrogenation process 失效
    脱氢工艺

    公开(公告)号：US20020072643A1

    公开(公告)日：2002-06-13

    申请号：US10074173

    申请日：2002-02-12

    Inventor： James R. Butler ,  James T. Merrill ,  Adrian M. Jacobsen

    IPC: C07C005/333 ,  C07C005/367

    CPC classification number: C07C5/333 ,  B01F5/06 ,  B01J8/0292 ,  B01J8/0453 ,  B01J8/065 ,  B01J2208/00061 ,  B01J2208/00212 ,  B01J2208/00548 ,  B01J2208/0084 ,  B01J2208/00849 ,  Y10S585/922 ,  Y10S585/923 ,  Y10S585/924 ,  C07C15/44 ,  C07C15/46

    Abstract: Process for the catalytic dehydrogenation of a C2 or C3 alkyl aromatic in which a feedstock containing the alkyl aromatic and steam is supplied into the inlet of a tubular reactor containing a dehydrogenation catalyst. Within the reactor, the feedstock flows through at least a portion of the reactor along a spiral flow path extending longitudinally of the reactor. The resulting vinyl aromatic product is then recovered from a downstream or outlet section of the reactor. The spiral flow path through which the feedstock is passed is located at least adjacent the inlet side of the reactor and at least a portion of the spiral flow path contains a particulate dehydrogenation catalyst. The spiral flow path may extend throughout a major portion of the elongated tubular reactor and may contain a particulate dehydrogenation catalyst in a substantial portion there. The feedstock containing the alkyl aromatic and steam is supplied into a plurality of tubular reactors located within the interior of a dehydrogenation reactor vessel and is arranged in a parallel relationship in which the tubular reactors are spaced laterally from one another and from the interior wall of the reaction vessel.

    Abstract translation: 将含有烷基芳族和蒸汽的原料供给到含有脱氢催化剂的管式反应器的入口中的C2或C3烷基芳族化合物的催化脱氢方法。 在反应器内，原料沿着反应器纵向延伸的螺旋流动路径流过反应器的至少一部分。 然后从反应器的下游或出口部分回收得到的乙烯基芳族化合物。 原料通过的螺旋流动路径至少位于反应器的入口侧，螺旋流路的至少一部分包含颗粒脱氢催化剂。 螺旋流动路径可以延伸穿过细长管式反应器的主要部分，并且可以在其中大部分含有颗粒状脱氢催化剂。 将含有烷基芳族化合物和蒸汽的原料供给到位于脱氢反应器容器内部的多个管式反应器中并且以平行关系排列，其中管式反应器彼此横向间隔开， 反应容器

    Inducing turbulent flow in catalyst beds
    9.
    发明申请
    Inducing turbulent flow in catalyst beds 审中-公开
    诱导催化剂床中的湍流

    公开(公告)号：US20020198429A1

    公开(公告)日：2002-12-26

    申请号：US10150850

    申请日：2002-05-16

    Applicant: Conoco Inc.

    Inventor： Sriram Ramani ,  Joe D. Allison ,  Richard Delgado

    IPC: C07C005/367 ,  C07C005/333 ,  B01J035/02

    CPC classification number: C10G2/33 ,  B01F5/064 ,  B01F5/0646 ,  B01F5/0647 ,  B01F5/065 ,  B01J19/2485 ,  B01J35/04 ,  C10G2/341

    Abstract: A catalyst bed is made of a monolith having a plurality of pores extending through the monolith, the pores forming tortuous flow paths through the monolith. The tortuous flow paths are obtained by modifying the monolith channels with turbulence-inducing objects or means. Catalyst is disposed on the wall surfaces formed by the pores. Reactants are passed through the tortuous flow paths creating turbulent flow thereby increasing the contact of the reactants with the catalyst on the wall surfaces and the mixing across the reactant stream.

    Abstract translation: 催化剂床由具有延伸穿过整料的多个孔的整料制成，孔形成通过整料的曲折的流动路径。 曲折的流动路径是通过用湍流诱导物体或装置修改整体通道获得的。 催化剂设置在由孔形成的壁表面上。 反应物通过曲折的流动路径，产生湍流，从而增加反应物与壁上的催化剂的接触以及反应物流的混合。

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