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    Aromatization process utilizing a pillared layered silicate plus a base metal or noble metal
    1.
    发明授权
    Aromatization process utilizing a pillared layered silicate plus a base metal or noble metal 失效
    使用柱状分层硅酸盐加贱金属或贵金属的芳构化方法

    公开(公告)号：US5008481A

    公开(公告)日：1991-04-16

    申请号：US459212

    申请日：1989-12-29

    Applicant: Ivy D. Johnson ,  Pochen Chu ,  Charles T. Kresge

    Inventor： Ivy D. Johnson ,  Pochen Chu ,  Charles T. Kresge

    IPC: C07C5/367 ,  C07C5/41

    CPC classification number: C07C5/415 ,  C07C5/367 ,  C07C5/417

    Abstract: There is provided a process for the aromatization of non-aromatic hydrocarbons having at least six carbon atoms. The non-aromatic feed is contacted with a catalyst which includes a base metal or noble metal which is incorporated into or onto a pillared layered silicate. A preferred pillared layered silicate is kenyaite containing interspathic silica, and a preferred base metal or noble metal is chromium.

    Abstract translation: 提供了一种使具有至少6个碳原子的非芳族烃芳构化的方法。 非芳族进料与催化剂接触，催化剂包括引入到柱状层状硅酸盐中或其上的贱金属或贵金属。 优选的柱状层状硅酸盐是含有间隙二氧化硅的肯尼亚，优选的贱金属或贵金属是铬。

    Dehydrogenation process utilizing a pillared layered silicate plus a base metal or noble metal
    2.
    发明授权
    Dehydrogenation process utilizing a pillared layered silicate plus a base metal or noble metal 失效
    使用柱状层状硅酸盐加贱金属或贵金属的脱氢方法

    公开(公告)号：US4956517A

    公开(公告)日：1990-09-11

    申请号：US459215

    申请日：1989-12-29

    Applicant: Ivy D. Johnson ,  Pochen Chu ,  Charles T. Kresge

    Inventor： Ivy D. Johnson ,  Pochen Chu ,  Charles T. Kresge

    IPC: C07C5/32 ,  C07C5/333

    CPC classification number: C07C5/325 ,  C07C5/3337

    Abstract: There is provided a process for the dehydrogenation of saturated hydrocarbons having from 2 to 5 carbon atoms. The feed is contacted with a catalyst which includes a base metal or noble metal which is incorporated into or onto a pillared layered silicate. A preferred pillared layered silicate is kenyaite containing interspathic silica, and a preferred base metal or noble metal is chromium.

    Abstract translation: 提供了具有2至5个碳原子的饱和烃脱氢的方法。 进料与催化剂接触，催化剂包括引入到柱状层状硅酸盐中或其上的贱金属或贵金属。 优选的柱状层状硅酸盐是含有间隙二氧化硅的肯尼亚，优选的贱金属或贵金属是铬。

    Pillared layered silicate compositions containing pillars of silica and metal oxide and their preparation
    4.
    发明授权
    Pillared layered silicate compositions containing pillars of silica and metal oxide and their preparation 失效
    含有二氧化硅和金属氧化物柱的柱状层状硅酸盐组合物及其制备方法

    公开(公告)号：US4968652A

    公开(公告)日：1990-11-06

    申请号：US494910

    申请日：1990-03-09

    Applicant: Ivy D. Johnson ,  Pochen Chu

    Inventor： Ivy D. Johnson ,  Pochen Chu

    IPC: B01J20/12 ,  B01J29/04 ,  C01B33/20

    CPC classification number: B01J29/049 ,  C01B33/20 ,  C01B33/28

    Abstract: Pillared layered silicate compositions containing pillars of silica and metal oxides, e.g., alumina are prepared by contacting organic-swelled layered silicates, e.g. kenyaite-type materials, with a hydrolyzable silica precursor, e.g., tetraethylorthosilicate which forms silanol groups between the layers and contacting the resulting product with an aqueous solution containing inorganic metal salt and effecting hydrolysis of the silanol groups.

    Abstract translation: 包含二氧化硅和金属氧化物柱的例如氧化铝的柱状层状硅酸盐组合物通过使有机溶胀的层状硅酸盐例如氧化铝接触而制备。 碱土金属类材料与可水解的二氧化硅前体，例如四乙基原硅酸盐，其在层之间形成硅烷醇基团，并使得到的产物与含有无机金属盐的水溶液接触并进行硅烷醇基团的水解。

    Production of ethylbenzene
    5.
    发明授权
    Production of ethylbenzene 失效
    生产乙苯

    公开(公告)号：US5334795A

    公开(公告)日：1994-08-02

    申请号：US967954

    申请日：1992-10-27

    Applicant: Pochen Chu ,  Michael E. Landis ,  Quang N. Le

    Inventor： Pochen Chu ,  Michael E. Landis ,  Quang N. Le

    IPC: C07C2/66

    CPC classification number: C07C2/66 ,  C07C2529/70

    Abstract: Ethylbenzene is produced by the alkylation of benzene with ethylene in the presence of an alkylation catalyst having a particular structure defined by its X-ray diffraction pattern. A preferred catalyst is the zeolite MCM-22. The process is typically carried out at a temperature of 300.degree. to 1000.degree. F. but the catalyst provides sufficient activity for the reaction to be carried out at temperatures below 700.degree. F. Liquid phase operation is preferred, giving a lower yield of polyethylated products. The use of the selected catalyst also results in a reduction of the xylene impurity level to values below 500 ppm in the product.

    Abstract translation: 在具有由其X射线衍射图形定义的特定结构的烷基化催化剂存在下，通过苯与乙烯的烷基化生产乙苯。 优选的催化剂是沸石MCM-22。 该方法通常在300至1000°F的温度下进行，但催化剂提供足够的活性以使反应在低于700°F的温度下进行。液相操作是优选的，从而降低聚乙烯化产物的产率 。 使用所选择的催化剂还导致二甲苯杂质水平降低到产品中低于500ppm的值。

    Layered cracking catalyst and method of manufacture and use thereof
    6.
    发明授权
    Layered cracking catalyst and method of manufacture and use thereof 失效
    层状裂化催化剂及其制造方法和用途

    公开(公告)号：US5179054A

    公开(公告)日：1993-01-12

    申请号：US735225

    申请日：1991-07-24

    Applicant: Paul H. Schipper ,  Hartley Owen ,  Joseph A. Herbst ,  Garry W. Kirker ,  Albin Huss, Jr. ,  Pochen Chu

    Inventor： Paul H. Schipper ,  Hartley Owen ,  Joseph A. Herbst ,  Garry W. Kirker ,  Albin Huss, Jr. ,  Pochen Chu

    IPC: B01J33/00 ,  C10G11/05

    CPC classification number: B01J33/00 ,  C10G11/05 ,  B01J2229/12 ,  B01J2229/42 ,  C10G2300/70

    Abstract: A layered catalyst suited to the catalytic cracking of heavy feeds comprises a core and a shell. The shell comprises at least 5 wt % of at least 1 molecular sieve having openings of at least 8 angstroms. The core comprises at least 10 wt % of at least 1 molecular sieve having openings comprising a 12 or less-membered ring and has a reduced, if any, content of said molecular sieve having openings of at least 8 angstroms, relative to its concentration in the shell. Suitable molecular sieve materials having openings of at least 8 angstroms include MCM-41, VPI-5, MCM-9 and layered metal oxides, e.g., pillared clays. The required molecular sieve of the core can include zeolite Y, Ultrastable Y or intermediate pore size zeolites such as ZSM-5. The shell which may further contain a metals passivator can act as a metals sink, and can remove metals from the unit by attrition. The catalyst is preferably prepared by forming the core and then coating or encapsulating the core with a shell material. The shell may also comprise an attritable coating of an amorphous rare earth oxide, aluminum oxide and aluminum phosphate composite, which traps metals.

    Abstract translation: 适用于重料的催化裂化的层状催化剂包括核和壳。 该壳包含至少5重量％的具有至少8埃的开口的至少1个分子筛。 核心包含至少10重量％的具有包含12个或更少元环的开口的至少1个分子筛，并且具有至少8埃的开口的所述分子筛的含量降低（如果有的话），相对于其浓度 贝壳。 具有至少8埃开口的合适的分子筛材料包括MCM-41，VPI-5，MCM-9和层状金属氧化物，例如柱状粘土。 核心所需的分子筛可包括沸石Y，超稳定Y或中等孔径沸石如ZSM-5。 可以进一步包含金属钝化剂的壳体可以用作金属沉槽，并且可以通过磨损从单元中去除金属。 催化剂优选通过形成核心然后用壳材料涂覆或包封核心来制备。 外壳还可以包含捕获金属的无定形稀土氧化物，氧化铝和磷酸铝复合材料的可磨损涂层。

    Zeolite-clay composition and uses thereof
    7.
    发明授权
    Zeolite-clay composition and uses thereof 失效

    公开(公告)号：US5140949A

    公开(公告)日：1992-08-25

    申请号：US758668

    申请日：1991-09-12

    Applicant: Pochen Chu ,  William E. Garwood

    Inventor： Pochen Chu ,  William E. Garwood

    IPC: A23K1/175 ,  B01J20/16 ,  B01J20/18

    CPC classification number: B01J20/18 ,  A23K20/28 ,  B01J20/16

    Abstract: A hydrous aluminosilicate adsorbent composition in which the active adsorbent is a mixture of non-fibrous clay with non-fibrous zeolite. The composition is useful as a feed supplement in animal husbandry, and as a topical adsorbent for veterinary use. The mixture has a high capacity for adsorption of ammonium cations, and a synergistically high selectivity for their adsorption. Beneficial effects as feed supplement may arise from lowering the amount of ammonia passed to the liver from the alimentary canal.

    Metal passivating agents
    9.
    发明授权
    Metal passivating agents 失效
    金属钝化剂

    公开(公告)号：US4919787A

    公开(公告)日：1990-04-24

    申请号：US335069

    申请日：1989-04-07

    Applicant: Arthur W. Chester ,  Pochen Chu ,  Albin Huss, Jr. ,  Garry W. Kirker

    Inventor： Arthur W. Chester ,  Pochen Chu ,  Albin Huss, Jr. ,  Garry W. Kirker

    IPC: B01J33/00 ,  C10G11/05

    CPC classification number: B01J33/00 ,  C10G11/05 ,  B01J2229/12 ,  B01J2229/42 ,  C10G2300/70 ,  Y10S502/521

    Abstract: An improved method for passivating metals in a hydrocarbon feedstock during catalytic cracking has been discovered. The method involves contacting the feedstock with a passivating agent comprising a precipitated porous rare earth oxide, alumina, and aluminum phosphate precipitate. The passivating agent may be coated on a cracking catalyst, be part of the matrix of a cracking catalyst, or be added to the cracking operation as discrete particles.

    Abstract translation: 已经发现了一种在催化裂化过程中钝化烃原料中的金属的改进方法。 该方法包括使原料与包含沉淀的多孔稀土氧化物，氧化铝和磷酸铝沉淀物的钝化剂接触。 钝化剂可以涂覆在裂化催化剂上，作为裂化催化剂的基质的一部分，或作为离散颗粒加入到裂化操作中。

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