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公开(公告)号：US08703830B2
公开(公告)日：2014-04-22
申请号：US13503481
申请日：2010-10-25
IPC分类号： C07C27/00
CPC分类号： B01J23/745 , B01J21/04 , B01J21/185 , B01J23/8892 , B01J27/224 , B01J35/1014 , B01J35/1019 , B01J35/1038 , B01J35/1042 , B01J37/0201 , B01J37/0203 , B01J37/0211 , B01J37/035 , B82Y30/00 , C07C1/044 , C07C1/0445 , C07C2521/04 , C07C2521/18 , C07C2523/745 , C10G2300/1022 , C10G2300/4006 , C10G2400/20 , Y02P30/40 , C07C11/02
摘要： Disclosed is a process for the production of lower olefins by the conversion of a feed stream comprising carbon monoxide and hydrogen, and catalysts as used therein, such as a Fischer-Tropsch process. By virtue of the invention, lower olefins can be formed from synthesis gas, with high selectivity, and low production of methane. The catalysts used herein comprise an α-alumina support, and a catalytically active component that comprises iron-containing particles dispersed onto the support in at least 1 wt. %. The majority of the iron-containing particles is in direct contact with the α-alumina and is well-distributed thereon. Preferably, the iron-containing particles have an average particle size below 30 nm, and most preferably below 10 nm. The supported catalysts not only show a high selectivity, but also a high catalyst activity and chemical and mechanical stability.
摘要翻译： 公开了通过转化包含一氧化碳和氢气的进料流以及如其中所用的催化剂如费 - 托方法生产低级烯烃的方法。 根据本发明，可以通过合成气体形成低级烯烃，具有高选择性和低甲烷生产能力。 本文使用的催化剂包含α-氧化铝载体和催化活性组分，其包含分散在载体上的含铁颗粒至少1重量％ ％。 大多数含铁颗粒与α-氧化铝直接接触并且分布良好。 优选地，含铁颗粒的平均粒径低于30nm，最优选低于10nm。 负载催化剂不仅显示出高选择性，而且具有高催化剂活性和化学和机械稳定性。
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公开(公告)号：US5720901A
公开(公告)日：1998-02-24
申请号：US361359
申请日：1994-12-21
CPC分类号： C01B3/40 , C01B3/386 , C01B2203/1011 , C01B2203/1023 , C01B2203/1029 , C01B2203/1047 , C01B2203/1064 , C01B2203/1082 , Y02P20/52
摘要： This invention concerns a process for the catalytic partial oxidation of a hydrocarbon feedstock. The process comprises contacting a feed mixture comprising the hydrocarbon feedstock and an oxygen-containing gas, which feed mixture also comprises nitrogen, with a catalyst capable of catalyzing the partial oxidation of the hydrocarbon feedstock, wherein the feed mixture also comprises a sulfur-containing compound. This process allows sulfur-containing hydrocarbon feedstocks to be processed without first undergoing a sulfur removal treatment. Accordingly, a process for the preparation of carbon monoxide and/or hydrogen from a hydrocarbon feedstock comprises subjecting the hydrocarbon feedstock in a first stage to a catalytic partial oxidation process as described above and subjecting at least a portion of the product of the first stage in a second stage to a desulfurization process.
摘要翻译： 本发明涉及烃原料的催化部分氧化的方法。 该方法包括将包含烃原料的进料混合物和含氧气体（该进料混合物还包含氮气）与能够催化烃原料的部分氧化的催化剂接触，其中进料混合物还包含含硫化合物 。 该方法允许在不首先进行硫去除处理的情况下处理含硫烃原料。 因此，从烃原料制备一氧化碳和/或氢气的方法包括使第一阶段的烃原料经历如上所述的催化部分氧化方法，并将第一阶段的产物的至少一部分 脱硫过程的第二阶段。
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3.发明授权公开(公告)号：US09126876B2
公开(公告)日：2015-09-08
申请号：US14009224
申请日：2012-02-10
CPC分类号： C07C1/046 , B01J21/04 , B01J23/745 , B01J35/006 , B01J35/1009 , B01J35/1014 , C07C1/044 , C07C2521/04 , C07C2523/745 , C10G2/332 , C10G2300/4006 , C10G2300/4012 , C10G2300/708 , C10G2400/20 , Y02P20/52 , C07C11/04 , C07C11/06
摘要： Effect Fischer-Tropsch synthesis of lower olefins by converting a syngas feedstream at a temperature within a range of from 300° C. to no more than 400° C. using a supported, iron-based catalyst under a total system pressure of at least 2 megapascals with a volumetric ratio of hydrogen to carbon monoxide of at least 3:1 with markedly lower coking rates than attainable at a total system pressure of less than 2 megapascals.
摘要翻译： 通过使用负载型铁基催化剂，在至少为2的总体系压力下将合成气原料流在300℃至不超过400℃的温度范围内进行转化，从而降低了低碳烯烃的合成。 氢气与一氧化碳的体积比至少为3:1的兆帕，具有比在小于2兆帕的总系统压力下可获得的显着降低的焦化速率。
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公开(公告)号：US08263522B2
公开(公告)日：2012-09-11
申请号：US12439915
申请日：2007-08-14
申请人： Jelle Rudolf Anne Sietsma , Adrianus Jacobus Van Dillen , Petra Elisabeth De Jongh , Krijn Pieter De Jong
发明人： Jelle Rudolf Anne Sietsma , Adrianus Jacobus Van Dillen , Petra Elisabeth De Jongh , Krijn Pieter De Jong
CPC分类号： B01J29/0333 , B01J23/70 , B01J35/002 , B01J35/006 , B01J37/088 , B01J37/16 , B82Y30/00 , C01G1/02 , C01G53/04 , C01P2002/72 , C01P2004/03 , C01P2004/64 , C01P2004/84 , C07C209/48 , C10G2/332 , C10G45/06
摘要： A method for converting a supported metal nitrate into the corresponding supported metal oxide comprises heating the metal nitrate to effect its decomposition under a gas mixture that contains nitrous oxide and has an oxygen content of
摘要翻译： 将负载的金属硝酸盐转化成相应的负载金属氧化物的方法包括加热金属硝酸盐以在含有一氧化二氮并且氧含量<5体积％的气体混合物下进行分解。 该方法在支撑材料上提供非常高度分散的金属氧化物。 金属氧化物可用作催化剂或催化剂前体。
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公开(公告)号：US08178467B2
公开(公告)日：2012-05-15
申请号：US12158854
申请日：2006-11-17
申请人： Jelle Rudolf Anne Sietsma , Adrianus jacobus Van Dillen , Petra Elisabeth De Jongh , Krijn Pieter De Jong
发明人： Jelle Rudolf Anne Sietsma , Adrianus jacobus Van Dillen , Petra Elisabeth De Jongh , Krijn Pieter De Jong
IPC分类号： B01J21/00
CPC分类号： C01G1/02 , B01J21/04 , B01J21/08 , B01J23/70 , B01J23/75 , B01J23/755 , B01J29/0333 , B01J35/006 , B01J35/0066 , B01J37/088 , B01J37/12 , B01J37/16 , B82Y30/00 , C01B13/18 , C01G3/02 , C01G3/08 , C01G49/02 , C01G51/04 , C01G53/04 , C01P2002/72 , C01P2004/04 , C01P2004/64 , C01P2006/12 , C01P2006/14 , C10G2/332 , C10G2/333 , C10G2/334 , C10G3/45 , C10G3/46 , C10G45/48 , C11C3/123 , Y02P30/20
摘要： A method for converting a supported metal nitrate into the corresponding supported metal oxide comprises heating the metal nitrate to effect its decomposition under a gas mixture that contains nitric oxide and has an oxygen content of
摘要翻译： 将负载的金属硝酸盐转化为相应的负载金属氧化物的方法包括加热金属硝酸盐，以在含有一氧化氮并且氧含量<5体积％的气体混合物下进行分解。 该方法在支撑材料上提供非常高度分散的金属氧化物。 金属氧化物可用作催化剂或催化剂前体。
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公开(公告)号：US20100099553A1
公开(公告)日：2010-04-22
申请号：US12439915
申请日：2007-08-14
申请人： Jelle Rudolf Anne Sietsma , Andrianus Jacobus Van Dillen , Petra Elisabeth De Jongh , Krijn Pieter De Jong
发明人： Jelle Rudolf Anne Sietsma , Andrianus Jacobus Van Dillen , Petra Elisabeth De Jongh , Krijn Pieter De Jong
IPC分类号： B01J21/08 , B01J23/755
CPC分类号： B01J29/0333 , B01J23/70 , B01J35/002 , B01J35/006 , B01J37/088 , B01J37/16 , B82Y30/00 , C01G1/02 , C01G53/04 , C01P2002/72 , C01P2004/03 , C01P2004/64 , C01P2004/84 , C07C209/48 , C10G2/332 , C10G45/06
摘要： A method for converting a supported metal nitrate into the corresponding supported metal oxide comprises heating the metal nitrate to effect its decomposition under a gas mixture that contains nitrous oxide and has an oxygen content of
摘要翻译： 将负载的金属硝酸盐转化成相应的负载金属氧化物的方法包括加热金属硝酸盐以在含有一氧化二氮并且氧含量<5体积％的气体混合物下进行分解。 该方法在支撑材料上提供非常高度分散的金属氧化物。 金属氧化物可用作催化剂或催化剂前体。
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7.发明申请PROCESS FOR PREPARING COMPOSITES COMPRISING CARBON AND MAGNESIUM FOR HYDROGEN STORAGE 审中-公开用于制备包含碳氢化合物和氢氧化物储存的复合材料的方法公开(公告)号：US20090289222A1
公开(公告)日：2009-11-26
申请号：US12307819
申请日：2007-07-06
申请人： Rudy Wilhelmus Peter Wagemans , Bibiana Sibbeltje Dauvillier , Petra Elisabeth De Jongh , Adrianus Jacobus Van Dillen , Krijn Pieter De Jong
发明人： Rudy Wilhelmus Peter Wagemans , Bibiana Sibbeltje Dauvillier , Petra Elisabeth De Jongh , Adrianus Jacobus Van Dillen , Krijn Pieter De Jong
CPC分类号： B01J20/20 , B01J20/02 , B01J20/04 , B01J20/28078 , B01J20/28097 , B01J20/3078 , B01J20/3204 , B01J20/3236 , B22F2998/00 , B22F2998/10 , B22F2999/00 , B82Y30/00 , C01B3/0021 , C01B3/0078 , C22C1/1005 , C22C1/1036 , C22C23/00 , C22C29/005 , C22C32/0084 , C22C2202/04 , Y02E60/325 , Y02E60/327 , Y10T428/13 , Y10T428/256 , Y10T428/30 , B22F2201/016 , C22C1/1094 , B22F2201/013
摘要： A process for preparing carbon and magnesium including composites, includes: a) contacting a carbon material including pores of which at least 30%, based on the total number of pores, have a pore diameter in the range 0.1 to 10×10−9 m with a molten metallic magnesium or magnesium alloy to obtain a intermediate composite; and b) cooling the intermediate composite to obtain a carbon and magnesium including composite. Also described is a carbon and magnesium including composite obtainable by the process of the invention, the use of a carbon and magnesium including composite obtainable by the process and a hydrogen storage system.
摘要翻译： 包括复合材料的制备碳和镁的方法包括：a）使包含孔的碳材料与基于总孔数的至少30％的孔径接触，其孔径在0.1至10×10 -9 m范围内， 熔融金属镁或镁合金，得到中间复合材料; 和b）冷却中间复合材料以获得包括复合材料的碳和镁。 还描述了通过本发明的方法获得的包含复合材料的碳和镁，包括通过该方法获得的包含复合材料的碳和镁和氢储存系统的用途。
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8.发明授权Modified Y-type zeolites having a trimodal intracrystalline structure, method for making same, and use thereof 有权具有三峰晶体结构的改性Y型沸石，其制备方法及其用途公开(公告)号：US09126183B2
公开(公告)日：2015-09-08
申请号：US13141281
申请日：2009-12-22
申请人： Sander Van Donk , Maxime Lacroix , Régine Kenmogne-Gatchuissi , François Fajula , Métin Bulut , Jean-Pierre Dath , Krijn Pieter De Jong , Petra Elisabeth De Jongh , Jovana Zecevic , Adrianus Nicolaas Cornelis Van Laak
发明人： Sander Van Donk , Maxime Lacroix , Régine Kenmogne-Gatchuissi , François Fajula , Métin Bulut , Jean-Pierre Dath , Krijn Pieter De Jong , Petra Elisabeth De Jongh , Jovana Zecevic , Adrianus Nicolaas Cornelis Van Laak
CPC分类号： B01J29/084 , B01J29/126 , B01J2229/16 , B01J2229/18 , B01J2229/20 , B01J2229/22 , B01J2229/38 , B01J2229/40 , B01J2229/42 , C01B39/026 , C01B39/24 , C10G47/16
摘要： The invention relates to a Y-type zeolite having a modified faujasite structure, the intracrystalline structure of which includes at least one network of micropores, at least one network of small mesopores having an average diameter ranging from 2 to 5 nm, and at least one network of large mesopores having an average diameter ranging from 10 to 50 nm. The invention also relates to particles including such zeolites and to the use thereof in a method for processing crude oil, particularly as a hydrocracking catalyst.
摘要翻译： 本发明涉及具有改性的八面沸石结构的Y型沸石，其结晶结构包括至少一个微孔网络，至少一个平均直径范围为2-5nm的小介孔网络，以及至少一个 具有10至50nm平均直径的大介孔的网络。 本发明还涉及包括这种沸石的颗粒以及其在用于加工原油，特别是加氢裂化催化剂的方法中的用途。
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公开(公告)号：US20120259026A1
公开(公告)日：2012-10-11
申请号：US13503481
申请日：2010-10-25
CPC分类号： B01J23/745 , B01J21/04 , B01J21/185 , B01J23/8892 , B01J27/224 , B01J35/1014 , B01J35/1019 , B01J35/1038 , B01J35/1042 , B01J37/0201 , B01J37/0203 , B01J37/0211 , B01J37/035 , B82Y30/00 , C07C1/044 , C07C1/0445 , C07C2521/04 , C07C2521/18 , C07C2523/745 , C10G2300/1022 , C10G2300/4006 , C10G2400/20 , Y02P30/40 , C07C11/02
摘要： Disclosed is a process for the production of lower olefins by the conversion of a feed stream comprising carbon monoxide and hydrogen, and catalysts as used therein, such as a Fischer-Tropsch process. By virtue of the invention, lower olefins can be formed from synthesis gas, with high selectivity, and low production of methane. The catalysts used herein comprise an α-alumina support, and a catalytically active component that comprises iron-containing particles dispersed onto the support in at least 1 wt. %. The majority of the iron-containing particles is in direct contact with the α-alumina and is well-distributed thereon. Preferably, the iron-containing particles have an average particle size below 30 nm, and most preferably below 10 nm. The supported catalysts not only show a high selectivity, but also a high catalyst activity and chemical and mechanical stability.
摘要翻译： 公开了通过转化包含一氧化碳和氢气的进料流以及如其中所用的催化剂如费 - 托方法生产低级烯烃的方法。 根据本发明，可以通过合成气体形成低级烯烃，具有高选择性和低甲烷生产能力。 本文使用的催化剂包含α-氧化铝载体和催化活性组分，其包含分散在载体上的含铁颗粒至少1重量％ ％。 大多数含铁颗粒与α-氧化铝直接接触并且分布良好。 优选地，含铁颗粒的平均粒径低于30nm，最优选低于10nm。 负载催化剂不仅显示出高选择性，而且具有高催化剂活性和化学和机械稳定性。
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10.发明申请MODIFIED Y-TYPE ZEOLITES HAVING A TRIMODAL INTRACRYSTALLINE STRUCTURE, METHOD FOR MAKING SAME, AND USE THEREOF 有权具有三角形结构结构的改性的Y型沸石，其制备方法及其用途公开(公告)号：US20120018349A1
公开(公告)日：2012-01-26
申请号：US13141281
申请日：2009-12-22
申请人： Sander Van Donk , Maxime Lacroix , Régine Kenmogne-Gatchuissi , François Fajula , Métin Bulut , Jean-Pierre Dath , Krijn Pieter De Jong , Petra Elisabeth De Jongh , Jovana Zecevic , Adrianus Nicolaas Cornelis Van Laak
发明人： Sander Van Donk , Maxime Lacroix , Régine Kenmogne-Gatchuissi , François Fajula , Métin Bulut , Jean-Pierre Dath , Krijn Pieter De Jong , Petra Elisabeth De Jongh , Jovana Zecevic , Adrianus Nicolaas Cornelis Van Laak
CPC分类号： B01J29/084 , B01J29/126 , B01J2229/16 , B01J2229/18 , B01J2229/20 , B01J2229/22 , B01J2229/38 , B01J2229/40 , B01J2229/42 , C01B39/026 , C01B39/24 , C10G47/16
摘要： The invention relates to a Y-type zeolite having a modified faujasite structure, the intracrystalline structure of which includes at least one network of micropores, at least one network of small mesopores having an average diameter ranging from 2 to 5 nm, and at least one network of large mesopores having an average diameter ranging from 10 to 50 nm. The invention also relates to particles including such zeolites and to the use thereof in a method for processing crude oil, particularly as a hydrocracking catalyst.
摘要翻译： 本发明涉及具有改性的八面沸石结构的Y型沸石，其结晶结构包括至少一个微孔网络，至少一个平均直径范围为2-5nm的小介孔网络，以及至少一个 具有10至50nm平均直径的大介孔的网络。 本发明还涉及包括这种沸石的颗粒以及其在用于加工原油，特别是加氢裂化催化剂的方法中的用途。
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