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    Azolyoxy-carboxylic acid amide compounds and herbicidal compositions
    1.
    发明授权
    Azolyoxy-carboxylic acid amide compounds and herbicidal compositions 失效
    芳氧基 - 羧酸酰胺化合物和除草组合物

    公开(公告)号：US4645525A

    公开(公告)日：1987-02-24

    申请号：US526518

    申请日：1983-08-26

    申请人： Heinz Forster ,  Wolfgang Hofer ,  Volker Mues ,  Ludwig Eue ,  Robert R. Schmidt

    发明人： Heinz Forster ,  Wolfgang Hofer ,  Volker Mues ,  Ludwig Eue ,  Robert R. Schmidt

    IPC分类号： A01N43/72 ,  A01N43/76 ,  A01N43/78 ,  A01N43/80 ,  A01N43/82 ,  A01N43/824 ,  A01N43/832 ,  A01N43/836 ,  A01N43/84 ,  A01N43/86 ,  A01N43/90 ,  C07D261/12 ,  C07D261/18 ,  C07D263/38 ,  C07D265/38 ,  C07D271/06 ,  C07D271/10 ,  C07D275/02 ,  C07D277/16 ,  C07D277/20 ,  C07D277/34 ,  C07D277/36 ,  C07D277/56 ,  C07D285/08 ,  C07D285/10 ,  C07D285/12 ,  C07D285/125 ,  C07D285/13 ,  C07D295/185 ,  C07D413/12 ,  C07D417/12 ,  C07D491/113

    CPC分类号： C07D295/185 ,  A01N43/80 ,  A01N43/82 ,  A01N43/90 ,  C07D277/34 ,  C07D277/56

    摘要： Azolyloxy-carboxylic acid amides of the formula ##STR1## wherein R is a five-membered hetero-aromatic monocyclic radical which contains an oxygen atom or a sulfur atom and 1 to 3 nitrogen atoms; orR is said monocyclic radical substituted by halogen, nitro, cyano, amino, alkylamino, dialkylamino, arylamino, alkylcarbonylamino, alkylcarbonyl, carboxyl, alkoxycarbonyl, carbamoyl, alkylaminocarbonyl, dialkylaminocarbonyl, arylaminocarbonyl substituted arylaminocarbonyl wherein the substituents are halogen, nitro or alkyl, aryl, substituted aryl wherein the substituents are halogen, nitro, cyano, alkyl, halogenoalkyl or alkoxy, aralkyl, haloaralkyl, alkoxy, halo-alkoxy, alkenoxy, alkynoxy, alkoxycarbonylalkoxy, aralkoxy or aryloxy, optionally halogen-substituted alkylthio, alkenylthio, alkynylthio, alkoxycarbonylalkylthio, aralkylthio, arylthio, alkylsulphinyl or alkylsulphonyl, optionally halogen-substituted alkyl, alkenyl, alkynyl, alkoxyalkyl, aralkoxyalkyl, aryloxyalkyl, alkylthioalkyl, alkylsulphinylalkyl, alkylsulphonylalkyl, arylthioalkyl, arylsulphinylalkyl, arylsulphonylalkyl, carboxyalkyl, alkoxycarbonylalkyl, optionally substituted aminocarbonylalkyl, cyanoalkyl or cycloalkyl,R.sup.1 is hydrogen or alkyl andR.sup.2 and R.sup.3 are individually selected from hydrogen, optionally substituted alkyl, alkenyl, alkynyl, aralkyl, cycloalkyl or aryl, or a nitrogen-containing heterocyclic radical, orR.sup.2 and R.sup.3, together with the nitrogen atom to which they are bonded, represent an optionally substituted, optionally partially unsaturated and optionally benzo-fused monocyclic or bicyclic radical which optionally contains one or more further hetero-atoms; are effective herbicides.

    摘要翻译： 式（I）的酰氧基 - 羧酸酰胺其中R是含有氧原子或硫原子和1-3个氮原子的五元杂芳族单环基团; 或R是被卤素，硝基，氰基，氨基，烷基氨基，二烷基氨基，芳基氨基，烷基羰基氨基，烷基羰基，羧基，烷氧基羰基，氨基甲酰基，烷基氨基羰基，二烷基氨基羰基，芳基氨基羰基取代的芳基氨基羰基取代的单环基团，其中取代基是卤素，硝基或烷基，芳基 其中取代基为卤素，硝基，氰基，烷基，卤代烷基或烷氧基，芳烷基，卤代烷基，烷氧基，卤代烷氧基，链烯氧基，炔氧基，烷氧羰基烷氧基，芳烷氧基或芳氧基，任选卤素取代的烷硫基，烯硫基，炔硫基，烷氧羰基烷硫基 ，芳烷硫基，芳硫基，烷基亚磺酰基或烷基磺酰基，任选卤素取代的烷基，烯基，炔基，烷氧基烷基，芳烷氧基烷基，芳氧基烷基，烷硫基烷基，烷基亚磺酰基烷基，烷基磺酰基烷基，芳硫基烷基，芳基亚磺酰基烷基，芳基磺酰基烷基，羧基烷基，烷氧基羰基烷基，任选取代的氨基羰基烷基，氰基烷基或环 烷基，R 1是氢或烷基，R 2和R 3分别选自氢，任选取代的烷基，烯基，炔基，芳烷基，环烷基或芳基或含氮杂环基，或者R 2和R 3与氮原子一起 它们被键合，表示任选地被任意取代的，任选地部分不饱和的和任选地苯并稠合的单环或双环基，其任选地含有一个或多个另外的杂原子; 是有效的除草剂。

    2-Substituted benzazole pesticide synergists
    2.
    发明授权
    2-Substituted benzazole pesticide synergists 失效
    2-取代的苯唑农药增效剂

    公开(公告)号：US4328219A

    公开(公告)日：1982-05-04

    申请号：US129853

    申请日：1980-03-12

    申请人： Volker Mues ,  Wolfgang Behrenz

    发明人： Volker Mues ,  Wolfgang Behrenz

    IPC分类号： A01N43/78 ,  A01N43/74 ,  A01N43/76 ,  C07D263/58 ,  C07D277/68

    CPC分类号： A01N43/74

    摘要： 2-Substituted benzazoles of the formula ##STR1## in which R represents optionally substituted alkyl, alkenyl, alkynyl, cycloalkyl, optionally substituted aryl or optionally substituted aralkyl,R.sup.1, R.sup.2, R.sup.3 and R.sup.4 independently of one another represent hydrogen, halogen, optionally halogen-substituted alkyl, optionally halogen-substituted alkoxy, nitro, cyano, alkylcarbonyl or alkoxycarbonyl, or two radicals in combination form a benzo radical,X and Y independently of one another represent oxygen or sulphur andn represents zero or 1,synergize conventional pesticides. Those benzazoles in whichR is --CH.sub.2 --C.dbd..tbd.CH,R.sup.1, R.sup.2, R.sup.3 and R.sup.4 represent independently of one another hydrogen or halogen (preferably chlorine),Y represents oxygen andn represents 1,are new and exhibit particularly high synergistic activity.

    摘要翻译： 其中R表示任选取代的烷基，烯基，炔基，环烷基，任选取代的芳基或任选取代的芳烷基，R 1，R 2，R 3和R 4彼此独立的2-取代的苯并唑代表氢，卤素，任选的卤素 取代的烷基，任选的卤素取代的烷氧基，硝基，氰基，烷基羰基或烷氧基羰基，或两个组合形成苯并基，X和Y彼此独立地表示氧或硫，n表示0或1，协同常规农药。 其中R为-CH 2 -C = 3BOND CH，R 1，R 2，R 3和R 4的那些苯并唑相互独立地表示氢或卤素（优选氯），Y表示氧且n表示1，表现出特别高的协同作用 。

    Combating arthropods with ferrocene-containing synergistic compositions
    5.
    发明授权
    Combating arthropods with ferrocene-containing synergistic compositions 失效
    将节肢动物与含有二茂铁的协同组合物相结合

    公开(公告)号：US4206227A

    公开(公告)日：1980-06-03

    申请号：US882824

    申请日：1978-03-02

    申请人： Volker Mues ,  Wolfgang Behrenz

    发明人： Volker Mues ,  Wolfgang Behrenz

    IPC分类号： A01N31/04 ,  A01N35/06 ,  A01N35/08 ,  A01N37/34 ,  A01N55/02 ,  A01N57/00 ,  A01N9/02

    CPC分类号： A01N55/02

    摘要： An arthropodicidal composition containing, as active ingredients, an arthropodicidally effective amount of (1) at least one ferrocene derivative of the formula ##STR1## in which R and R.sup.1 each independently is hydrogen, an alkyl or alkenyl radical optionally substituted by alkoxycarbonyl, aralkyl, cyanoalkyl, nitrile, or ##STR2## R.sup.2 is hydrogen, optionally substituted alkyl, optionally substituted cycloalkyl, optionally substituted phenyl or alkoxy,R.sup.3 is hydrogen, alkyl, alkanoyl or a polyalkylene polyether group,R.sup.4 and R.sup.5 each independently is alkyl or together are an alkylene radical,X is oxygen, hydroxyimino or alkoxyimino and,Y is oxygen or sulphur,and (2) at least one compound selected from (A) carbamates, (B) carboxylic acid esters, including the natural and synthetic pyrethroids, (C) phosphoric acid esters, (D) cycloalkanes, (E) halogenoalkanes and (F) tin compounds.

    摘要翻译： 一种节肢动物杀伤组合物，其含有作为活性成分的节肢动物节肢动物有效量的（1）至少一种下式的二茂铁衍生物，其中R和R 1各自独立地为氢，任选被烷氧基羰基，芳烷基取代的烷基或烯基， 氰基烷基，腈或R 2是氢，任选取代的烷基，任选取代的环烷基，任选取代的苯基或烷氧基，R 3是氢，烷基，烷酰基或聚亚烷基聚醚基团，R 4和R 5各自独立地是烷基或一起是 亚烷基，X是氧，羟亚氨基或烷氧基亚氨基，Y是氧或硫，和（2）至少一种选自（A）氨基甲酸酯，（B）羧酸酯，包括天然和合成拟除虫菊酯的化合物，（C） 磷酸酯，（D）环烷烃，（E）卤代烷烃和（F）锡化合物。

    Fertilizers for supplying plants with iron
    6.
    发明授权
    Fertilizers for supplying plants with iron 失效
    供应植物铁的肥料

    公开(公告)号：US4167405A

    公开(公告)日：1979-09-11

    申请号：US865479

    申请日：1977-12-29

    申请人： Volker Mues ,  Johannes Niggemann

    发明人： Volker Mues ,  Johannes Niggemann

    IPC分类号： C05D9/02 ,  C07F15/02 ,  C07F17/02 ,  C05F11/00

    CPC分类号： C07F17/02 ,  C05D9/02 ,  Y10S71/02

    摘要： A method of supplying plants with iron which comprises applying to the plants, or to the substrate in which they grow, at least one ferrocene derivative of the formula ##STR1## wherein R represents alkyl with 3 to 20 carbon atoms, preferably 7 to 20 carbon atoms, alone or in admixture with a diluent or carrier.

    摘要翻译： 给植物提供铁的方法，其包括向植物或其生长的基质施用至少一种下式的二茂铁衍生物（I），其中R表示具有3至20个碳原子的烷基，优选7 至20个碳原子，单独或与稀释剂或载体混合。

    Substituted carboxylic acid amide herbicides
    7.
    发明授权
    Substituted carboxylic acid amide herbicides 失效
    取代的羧酸酰胺除草剂

    公开(公告)号：US4833243A

    公开(公告)日：1989-05-23

    申请号：US678076

    申请日：1984-12-04

    申请人： Heinz Forster ,  Wolfgang Hofer ,  Volker Mues ,  Ludwig Eue ,  Robert R. Schmidt

    发明人： Heinz Forster ,  Wolfgang Hofer ,  Volker Mues ,  Ludwig Eue ,  Robert R. Schmidt

    IPC分类号： C07D209/34 ,  A01N43/74 ,  A01N43/76 ,  A01N43/78 ,  A01P13/00 ,  C07D263/54 ,  C07D263/58 ,  C07D277/62 ,  C07D277/68 ,  C07D317/00 ,  C07D413/12 ,  C07D417/12 ,  C07D491/10 ,  C07D491/113 ,  C07D493/10 ,  C07D513/04

    CPC分类号： C07D277/68 ,  A01N43/74 ,  C07D493/10 ,  C07D513/04

    摘要： Novel substituted carboxylic acid amide herbicides of the formula ##STR1## wherein n is an integer from 1 to 4each R is independently selected from hydrogen, halogen, alkyl, haloalkyl, alkoxy, haloalkoxy, alkylthio, haloalkylthio, amino, alkylamino, dialkylamino, nitro cyano and alkoxycarbonyl; and two R radicals taken together can represent methylenedioxy, dichloromethylenedioxy or difluoromethylenedioxy,R.sup.1 is hydrogen or alkyl,R.sup.2 and R.sup.3 are individually selected from hydrogen or a radical selected from alkyl, alkenyl, alkynyl, aralkyl, cycloalkyl, aryl and nitrogen-containing heterocycles, each of which radicals may be substituted and each of which radicals may, together with the nitrogen atom to which they are attached, form an optionally substituted, optionally partially unsaturated and optionally benzo-fused monocyclic or bicyclic radical, which may contain one or more further hetero-atoms, andX is oxygen or sulfur.

    摘要翻译： 式（I）的新型取代的羧酸酰胺除草剂其中n是1至4的整数，每个R独立地选自氢，卤素，烷基，卤代烷基，烷氧基，卤代烷氧基，烷硫基，卤代烷硫基，氨基，烷基氨基， 二烷基氨基，硝基氰基和烷氧基羰基; 一起取代的二个R基团可以代表亚甲二氧基，二氯亚甲二氧基或二氟亚甲二氧基，R 1是氢或烷基，R 2和R 3分别选自氢或选自烷基，烯基，炔基，芳烷基，环烷基，芳基和含氮杂环的基团， 其中每个基团可以被取代，并且其中每个基团可以与它们所连接的氮原子一起形成任选取代的，任选地部分不饱和的和任选的苯并稠合的单环或双环基团，其可以含有一个或多个另外的基团 杂原子，X是氧或硫。

    Ferrocene derivative for supplying plants with iron
    10.
    发明授权
    Ferrocene derivative for supplying plants with iron 失效
    用于供应铁矿石的FERROCENE DERIVATIVE

    公开(公告)号：US4053296A

    公开(公告)日：1977-10-11

    申请号：US721736

    申请日：1976-09-09

    申请人： Volker Mues ,  Johannes Niggemann

    发明人： Volker Mues ,  Johannes Niggemann

    IPC分类号： C05D9/02 ,  C07F9/6518 ,  C07F15/02 ,  C07F17/02 ,  C05F11/10

    CPC分类号： C07F17/02 ,  C05D9/02 ,  Y10S71/02

    摘要： Ferrocene derivatives of the formula ##STR1## IN WHICH R represents the group COOR.sup.1,in whichR.sup.1 represents hydrogen, alkyl, one equivalent of an alkali metal, alkaline earth metal or heavy metal cation, or an ammonium cation in which one or moreHydrogen atoms can be replaced by alkyl,Or R represents the group COR.sup.2in whichR.sup.2 represents optionally substituted alkyl, optionally substituted alkenyl, optionally substituted cycloalkyl, optionally substituted cycloalkenyl or optionally substituted phenyl,OrR represents the group ##STR2## in which R.sup.3 represents hydrogen or alkyl andR.sup.4 represents a ureido or thioureido radical, a radical of the formula --CH.sub.2 --CH.sub.2 --N.dbd.CH--ferrocene, a 5-membered or 6-membered heterocyclic radical or a group of the formula --OR.sup.5 or --NH-R.sup.6,in whichR.sup.5 represents hydrogen, alkyl, one equivalent of an alkali metal or alkaline earth metal cation, or an ammonium cation in which one or more hydrogen atoms canbe replaced by alkyl, andR.sup.6 represents aryl or a 5-membered or 6-membered heterocyclic radical,OrR represents the sulfonamide group or the radical --SO.sub.3 R.sup.7,in whichR.sup.7 represents hydrogen, alkyl, one equivalent of an alkali metal or alkaline earth metal cation, or an ammonium cation in which one or more hydrogen atoms can be replaced by alkyl,Or p1 R represents an alkyl, aralkyl or aryl radical which can be substituted by hydroxyl, cyano, COOR.sup.1 or ##STR3## in which R.sup.1 has the above-mentioned meansing,R', r" and R'", independently of one another, each represent hydrogen or alkyl andA.sup.- represents halide or methosulfate, are outstandingly effective for supplying plants with the micro-nutrient iron.