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    Moving bed hydrocarbon conversion process
    2.
    发明授权
    Moving bed hydrocarbon conversion process 失效
    移动床碳氢化合物转化过程

    公开(公告)号：US5157181A

    公开(公告)日：1992-10-20

    申请号：US621692

    申请日：1990-12-03

    申请人： Laurence O. Stine ,  Howard E. Fullerton ,  Thomas R. Fritsch ,  Paul T. Barger

    发明人： Laurence O. Stine ,  Howard E. Fullerton ,  Thomas R. Fritsch ,  Paul T. Barger

    IPC分类号： B01J29/90 ,  C07C1/00 ,  C07C1/20 ,  C10G3/00 ,  C10L1/06

    CPC分类号： C07C1/00 ,  B01J29/90 ,  B01J8/12 ,  C07C1/20 ,  C10G3/49 ,  C10G3/55 ,  C10G3/62 ,  C10L1/06 ,  C07C2529/85 ,  C10G2400/20 ,  C10G2400/28 ,  Y02P20/52 ,  Y02P20/584

    摘要： Moving bed hydrocarbon conversion processes are disclosed wherein a carbonaceous material is deposited on a solid catalyst used in the conversion process to form a coked catalyst which is regenerated in a regeneration zone in order to remove the carbonaceous deposit material from the catalyst and provide a regenerated catalyst having an increased number of active catalyst sites relative to the coked catalyst. The regenerated catalyst is then added to the reaction zone at a rate effective to enhance the conversion to desired products without enhancing the conversion to undesired by-products. When a radial flow reaction zone is employed a relatively constant amount of active catalyst sites can be maintained through the reaction zone by increasing the thickness of annulus through which the catalyst flows in the lower section of the reaction zone wherein the catalyst is more severely coked and has fewer active catalyst sites. The conversion of aliphatic hetero compounds, such as methanol to produce olefins in the C.sub.2 -C.sub.4 carbon range is specifically exemplified.

    摘要翻译： 公开了移动床烃转化方法，其中碳质材料沉积在转化过程中使用的固体催化剂上以形成焦化催化剂，其在再生区再生，以便从催化剂中除去含碳沉积材料并提供再生催化剂 相对于焦化催化剂具有增加的活性催化剂位点数。 然后将再生的催化剂以有效增加转化成所需产物的速率加入到反应区中，而不增加转化为不需要的副产物。 当使用径向流动反应区时，通过增加催化剂在反应区的下部流动的环空的厚度，通过反应区可维持相对恒定量的活性催化剂位点，其中催化剂被更严重地焦化， 活性催化剂位点较少。 脂肪族杂化物如甲醇转化成C2-C4碳范围的烯烃。

    Oil Recovery by In-Situ Cracking and Hydrogenation
    3.
    发明申请
    Oil Recovery by In-Situ Cracking and Hydrogenation 失效
    通过原位开裂和氢化回收油

    公开(公告)号：US20100078172A1

    公开(公告)日：2010-04-01

    申请号：US12241707

    申请日：2008-09-30

    申请人： Laurence O. Stine ,  Paul T. Barger

    发明人： Laurence O. Stine ,  Paul T. Barger

    IPC分类号： E21B43/24

    CPC分类号： E21B43/24 ,  E21B43/243

    摘要： Enhanced recovery of crude oil from an oil well is provided by in-situ cracking of an oxygenated organic compound to form hydrogen. The crude oil is then hydrogenated and hydrogenation reaction products and crude oil are recovered from the oil well.

    摘要翻译： 通过原位裂解含氧有机化合物以形成氢，提供从油井中提高原油的回收率。 然后将原油氢化，从油井中回收氢化反应产物和原油。

    Sapo catalysts and use thereof in methanol conversion processes
    8.
    发明授权
    Sapo catalysts and use thereof in methanol conversion processes 失效
    Sapo催化剂及其在甲醇转化过程中的应用

    公开(公告)号：US5248647A

    公开(公告)日：1993-09-28

    申请号：US793874

    申请日：1991-12-23

    申请人： Paul T. Barger

    发明人： Paul T. Barger

    IPC分类号： B01J29/85 ,  C07C1/20

    CPC分类号： B01J29/85 ,  C07C1/20 ,  B01J2229/36 ,  B01J2229/40 ,  B01J2229/42 ,  C07C2529/85 ,  Y02P20/52 ,  Y02P30/42

    摘要： Hydrothermal treatment of silicoaluminophosphate molecular sieves at temperatures in excess of about 700.degree. C. for periods sufficient to destroy a large proportion of their acid sites while retaining at least 80 percent of their crystallinity is found to result in a catalyst for converting methanol to lower olefins having increased catalyst life, increased selectivity for C.sub.2 -C.sub.3 olefins and decreased selectivity for paraffin production than the untreated SAPO-n starting composition.

    摘要翻译： 在超过约700℃的温度下水热处理硅铝磷酸盐分子筛，足以破坏其大部分酸性位点同时保持其至少80％的结晶度的时间段被发现导致用于将甲醇转化为低级烯烃的催化剂 与未处理的SAPO-n起始组合物相比，催化剂寿命增加，C2-C3烯烃的选择性提高，石蜡生产的选择性降低。

    Process for converting methanol to olefins using an improved metal aluminophosphate catalyst
    9.
    发明授权
    Process for converting methanol to olefins using an improved metal aluminophosphate catalyst 失效
    使用改进的金属磷酸铝催化剂将甲醇转化为烯烃的方法

    公开(公告)号：US5191141A

    公开(公告)日：1993-03-02

    申请号：US862018

    申请日：1992-04-01

    申请人： Paul T. Barger ,  Stephen T. Wilson ,  Jennifer S. Holmgren

    发明人： Paul T. Barger ,  Stephen T. Wilson ,  Jennifer S. Holmgren

    IPC分类号： B01J29/84 ,  B01J29/85 ,  C07C1/20

    CPC分类号： B01J29/85 ,  B01J29/84 ,  C07C1/20 ,  B01J2229/26 ,  B01J2229/42 ,  C07C2529/83 ,  C07C2529/85 ,  Y02P20/52

    摘要： This invention relates to an improved process for converting methanol to light olefins using an ELAPO catalyst. The catalyst comprises a metal aluminophosphate molecular sieve having the empirical formula (EL.sub.x Al.sub.y P.sub.z)O.sub.2 where EL is a metal and x,y and z are mole fractions of EL, Al and P respectively. Preferred metals are silicon, magnesium and cobalt, with silicon especially preferred. The molecular sieve catalyst is composed of particles at least 50% of which have a particle size less than 1.0 .mu.m and no more than 10% of the particles have a particle size greater than 2.0 .mu.m. It is also preferred that the metal content (x) be from about 0.005 and 0.05 mole fraction.

    摘要翻译： 本发明涉及使用ELAPO催化剂将甲醇转化为轻质烯烃的改进方法。 催化剂包括具有经验式（ELxAlyPz）O 2的金属铝磷酸盐分子筛，其中EL是金属，x，y和z分别是EL，Al和P的摩尔分数。 优选的金属是硅，镁和钴，特别优选硅。 分子筛催化剂由至少50％的粒径小于1.0μm且不超过10％的颗粒具有大于2.0μm的粒度的颗粒组成。 金属含量（x）也优选为约0.005和0.05摩尔分数。

    Process for the isomerization of dimethylnaphthalenes
    10.
    发明授权
    Process for the isomerization of dimethylnaphthalenes 失效
    二甲基萘异构化的方法

    公开(公告)号：US4777312A

    公开(公告)日：1988-10-11

    申请号：US138249

    申请日：1987-12-28

    申请人： Steve T. Bakas ,  Paul T. Barger

    发明人： Steve T. Bakas ,  Paul T. Barger

    IPC分类号： B01J29/22 ,  C07C5/22 ,  C07C5/27 ,  C10G45/64

    CPC分类号： B01J29/22 ,  C07C5/2791 ,  Y02P20/582

    摘要： Superior isomerization performance is obtained in an isomerization process employing a catalytic composition comprising a Group VIII noble metal and a hydrogen form mordenite incorporated with alumina. The superior isomerization performance is achieved using a catalyst composition having a surface area of at least 580 m.sup.2 /g. A novel method of preparing an isomerization catalyst having a surface area of at least 580 m.sup.2 /g is characterized by contacting a formed catalytic composite with an acidic aqueous solution prior to addition of the Group VIII noble metal. The isomerization process is particularly useful in the isomerization of a dimethylnaphthalene containing feedstock into a product that contains a higher concentration of the 2,6-dimethylnaphthalene isomer than did the feedstock.

    摘要翻译： 在使用包含VIII族贵金属和与氧化铝结合的氢形式丝光沸石的催化组合物的异构化方法中获得了优异的异构化性能。 使用具有至少580m 2 / g的表面积的催化剂组合物来实现优异的异构化性能。 制备具有至少580m 2 / g的表面积的异构化催化剂的新方法的特征在于，在加入第VIII族贵金属之前，使形成的催化剂复合物与酸性水溶液接触。 异构化方法特别可用于将含二甲基萘的原料异构化成含有比原料更高浓度的2,6-二甲基萘异构体的产物。