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公开(公告)号：US07858667B2
公开(公告)日：2010-12-28
申请号：US11611160
申请日：2006-12-15
申请人： Jianli Hu , Robert A. Dagle , Jamelyn D. Holladay , Chunshe Cao , Yong Wang , James F. White , Douglas C. Elliott , Don J. Stevens
发明人： Jianli Hu , Robert A. Dagle , Jamelyn D. Holladay , Chunshe Cao , Yong Wang , James F. White , Douglas C. Elliott , Don J. Stevens
IPC分类号： C07C27/00
CPC分类号： C07C29/152 , B01J19/0093 , B01J2219/00835 , B01J2219/00873 , B01J2219/00961 , B01J2219/00984 , C07C29/157 , Y02P20/52 , C07C31/04 , C07C31/08 , C07C31/02
摘要： Methods for producing alcohols from CO or CO2 and H2 utilizing a palladium-zinc on alumina catalyst are described. Methods of synthesizing alcohols over various catalysts in microchannels are also described. Ethanol, higher alcohols, and other C2+ oxygenates can produced utilizing Rh—Mn or a Fisher-Tropsch catalyst.
摘要翻译： 描述了使用氧化铝催化剂上的钯 - 锌从CO或CO 2和H 2生产醇的方法。 还描述了在微通道中在各种催化剂上合成醇的方法。 可以使用Rh-Mn或Fisher-Tropsch催化剂生产乙醇，高级醇和其他C2 +含氧化合物。
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2.发明授权公开(公告)号：US07208136B2
公开(公告)日：2007-04-24
申请号：US10440448
申请日：2003-05-16
申请人： Jamelyn D. Holladay , Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Guanguang Xia , Eddie G. Baker , Daniel R. Palo , Max R. Phelps , Heon Jung
发明人： Jamelyn D. Holladay , Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Guanguang Xia , Eddie G. Baker , Daniel R. Palo , Max R. Phelps , Heon Jung
CPC分类号： C01B3/326 , B01J19/0093 , B01J21/04 , B01J23/60 , B01J35/002 , B01J37/0201 , B01J2219/00783 , B01J2219/00788 , B01J2219/00822 , B01J2219/00824 , B01J2219/00835 , B01J2219/00862 , B01J2219/00873 , B01J2219/00891 , B01J2219/00961 , B01J2219/00997 , C01B3/586 , C01B2203/0233 , C01B2203/0445 , C01B2203/047 , C01B2203/1041 , C01B2203/1064 , C01B2203/1223 , Y02P20/52
摘要： The present invention provides steam reforming catalyst compositions containing Pd and Zn, and methods of steam reforming alcohols over a catalyst. Surprisingly superior results and properties of the present invention, including low temperature activity and/or low carbon monoxide output, are also described. Methods of making a steam reforming catalyst are also provided.
摘要翻译： 本发明提供含有Pd和Zn的蒸汽重整催化剂组合物，以及在催化剂上蒸汽重整醇的方法。 还描述了包括低温活性和/或低一氧化碳输出的本发明的令人惊奇的优异结果和性质。 还提供了制备蒸汽重整催化剂的方法。
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3.发明授权Microcombustors, microreformers, and methods involving combusting or reforming fluids 有权微型燃烧器，微型重整器和涉及燃烧或重整流体的方法公开(公告)号：US07585472B2
公开(公告)日：2009-09-08
申请号：US10434443
申请日：2003-05-07
申请人： Jamelyn D. Holladay , Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Guanguang Xia , Eddie G. Baker , Daniel R. Palo , Max Phelps , Heon Jung
发明人： Jamelyn D. Holladay , Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Guanguang Xia , Eddie G. Baker , Daniel R. Palo , Max Phelps , Heon Jung
IPC分类号： B01J8/04
CPC分类号： F23C13/00 , B01J19/0093 , B01J21/04 , B01J21/066 , B01J23/60 , B01J23/63 , B01J37/03 , B01J2219/00783 , B01J2219/00833 , B01J2219/00835 , B01J2219/00873 , B01J2219/00891 , C01B3/323 , C01B3/384 , C01B2203/00 , C01B2203/0233 , C01B2203/04 , C01B2203/0445 , C01B2203/047 , C01B2203/066 , C01B2203/0811 , C01B2203/0816 , C01B2203/0822 , C01B2203/0827 , C01B2203/1011 , C01B2203/1052 , C01B2203/1064 , C01B2203/1076 , C01B2203/1082 , C01B2203/1217 , C01B2203/1223 , C01B2203/1288 , C01B2203/1619 , F23C2900/03001 , Y02P20/128 , Y02P20/52
摘要： The invention describes combustors and steam reformers and methods of combustion and steam reforming. For example, integrated combustion reactors are described in which heat from combustion is transferred to an endothermic reaction. Thermally efficient reactors and methods of alcohol steam reforming are also described. Also described is an integrated combustor/reformer containing a methanation catalyst.
摘要翻译： 本发明描述了燃烧器和蒸汽重整器以及燃烧和蒸汽重整的方法。 例如，描述了将来自燃烧的热转移到吸热反应的综合燃烧反应器。 还描述了热效率的反应器和醇蒸汽重整的方法。 还描述了含有甲烷化催化剂的一体化燃烧器/重整器。
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4.发明申请Microcombustors, Microreformers, And Methods Involving Combusting Or Reforming Liquids 有权微燃烧器，微型反应器和涉及燃烧或重整液体的方法公开(公告)号：US20090297435A1
公开(公告)日：2009-12-03
申请号：US12538140
申请日：2009-08-09
申请人： Jamelyn D. Holladay , Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Guanguang Xia , Eddie G. Baker , Daniel R. Palo , Max Phelps , Heon Jung
发明人： Jamelyn D. Holladay , Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Guanguang Xia , Eddie G. Baker , Daniel R. Palo , Max Phelps , Heon Jung
CPC分类号： F23C13/00 , B01J19/0093 , B01J21/04 , B01J21/066 , B01J23/60 , B01J23/63 , B01J37/03 , B01J2219/00783 , B01J2219/00833 , B01J2219/00835 , B01J2219/00873 , B01J2219/00891 , C01B3/323 , C01B3/384 , C01B2203/00 , C01B2203/0233 , C01B2203/04 , C01B2203/0445 , C01B2203/047 , C01B2203/066 , C01B2203/0811 , C01B2203/0816 , C01B2203/0822 , C01B2203/0827 , C01B2203/1011 , C01B2203/1052 , C01B2203/1064 , C01B2203/1076 , C01B2203/1082 , C01B2203/1217 , C01B2203/1223 , C01B2203/1288 , C01B2203/1619 , F23C2900/03001 , Y02P20/128 , Y02P20/52
摘要： The invention describes combustors and steam reformers and methods of combustion and steam reforming. For example, integrated combustion reactors are described in which heat from combustion is transferred to an endothermic reaction. Thermally efficient reactors and methods of alcohol steam reforming are also described. Also described is an integrated combustor/reformer containing a methanation catalyst.
摘要翻译： 本发明描述了燃烧器和蒸汽重整器以及燃烧和蒸汽重整的方法。 例如，描述了将来自燃烧的热转移到吸热反应的综合燃烧反应器。 还描述了热效率的反应器和醇蒸汽重整的方法。 还描述了含有甲烷化催化剂的一体化燃烧器/重整器。
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5.发明授权公开(公告)号：US07563390B2
公开(公告)日：2009-07-21
申请号：US11691400
申请日：2007-03-26
申请人： Jamelyn D. Holladay , Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Guanguang Xia , Eddie G. Baker , Daniel R. Palo , Max R. Phelps , Heon Jung
发明人： Jamelyn D. Holladay , Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Guanguang Xia , Eddie G. Baker , Daniel R. Palo , Max R. Phelps , Heon Jung
CPC分类号： C01B3/326 , B01J19/0093 , B01J21/04 , B01J23/60 , B01J35/002 , B01J37/0201 , B01J2219/00783 , B01J2219/00788 , B01J2219/00822 , B01J2219/00824 , B01J2219/00835 , B01J2219/00862 , B01J2219/00873 , B01J2219/00891 , B01J2219/00961 , B01J2219/00997 , C01B3/586 , C01B2203/0233 , C01B2203/0445 , C01B2203/047 , C01B2203/1041 , C01B2203/1064 , C01B2203/1223 , Y02P20/52
摘要： The present invention provides steam reforming catalyst compositions containing Pd and Zn, and methods of steam reforming alcohols over a catalyst. Surprisingly superior results and properties of the present invention, including low temperature activity and/or low carbon monoxide output, are also described. Methods of making a steam reforming catalyst are also provided.
摘要翻译： 本发明提供含有Pd和Zn的蒸汽重整催化剂组合物，以及在催化剂上蒸汽重整醇的方法。 还描述了包括低温活性和/或低一氧化碳输出的本发明的令人惊奇的优异结果和性质。 还提供了制备蒸汽重整催化剂的方法。
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公开(公告)号：US20090297434A1
公开(公告)日：2009-12-03
申请号：US12276341
申请日：2008-11-23
申请人： Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Chunshe Cao
发明人： Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Chunshe Cao
IPC分类号： C01B3/02
CPC分类号： B01J37/0205 , B01J23/60 , B01J37/0248 , C01B3/326 , C01B2203/0233 , C01B2203/1029 , C01B2203/1064 , C01B2203/1076 , C01B2203/1217 , C01B2203/1223 , Y02P20/52
摘要： The present invention provides catalysts, reactors, and methods of steam reforming alcohols over a catalyst. Surprisingly superior results and properties obtained in methods and catalysts of the present invention are also described.
摘要翻译： 本发明提供了在催化剂上蒸汽重整醇的催化剂，反应器和方法。 还描述了在本发明的方法和催化剂中获得的令人惊奇的优异结果和性能。
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公开(公告)号：US07470648B2
公开(公告)日：2008-12-30
申请号：US10076880
申请日：2002-02-13
申请人： Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Chunshe Cao
发明人： Yong Wang , Jianli Hu , Ya-Huei Chin , Robert A. Dagle , Chunshe Cao
IPC分类号： B01J23/02
CPC分类号： B01J37/0205 , B01J23/60 , B01J37/0248 , C01B3/326 , C01B2203/0233 , C01B2203/1029 , C01B2203/1064 , C01B2203/1076 , C01B2203/1217 , C01B2203/1223 , Y02P20/52
摘要： The present invention provides catalysts, reactors, and methods of steam reforming alcohols over a catalyst. Surprisingly superior results and properties obtained in methods and catalysts of the present invention are also described.
摘要翻译： 本发明提供了在催化剂上蒸汽重整醇的催化剂，反应器和方法。 还描述了在本发明的方法和催化剂中获得的令人惊奇的优异结果和性能。
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8.发明授权Methods of producing hydrogen via the water-gas shift reaction over a Pd-Zn catalyst 有权通过Pd-Zn催化剂通过水煤气变换反应生产氢气的方法公开(公告)号：US07758846B2
公开(公告)日：2010-07-20
申请号：US11305840
申请日：2005-12-16
申请人： Robert A. Dagle , Yong Wang , Jianli Hu
发明人： Robert A. Dagle , Yong Wang , Jianli Hu
CPC分类号： C01B3/16 , B01J19/0093 , B01J23/60 , B01J37/0201 , B01J2219/00783 , B01J2219/00788 , B01J2219/00826 , B01J2219/00835 , B01J2219/0086 , B01J2219/00867 , B01J2219/00873 , C01B2203/0283 , C01B2203/1029 , C01B2203/1035 , C01B2203/1064 , C01B2203/1076 , Y02P20/52
摘要： Methods for producing hydrogen via the water-gas shift reaction utilizing a palladium-zinc on alumina catalyst are described.
摘要翻译： 描述了使用氧化铝催化剂上的钯 - 锌通过水煤气变换反应生产氢的方法。
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公开(公告)号：US08957259B2
公开(公告)日：2015-02-17
申请号：US11241321
申请日：2005-09-30
申请人： Robert A. Dagle , Yong Wang , Eddie G. Baker , Jianli Hu
发明人： Robert A. Dagle , Yong Wang , Eddie G. Baker , Jianli Hu
CPC分类号： C07C41/09 , C07C41/01 , C07C43/043
摘要： Disclosed are methods for producing dimethyl ether (DME) from methanol and for producing DME directly from syngas, such as syngas from biomass. Also disclosed are apparatus for DME production. The disclosed processes generally function at higher temperatures with lower contact times and at lower pressures than conventional processes so as to produce higher DME yields than do conventional processes. Certain embodiments of the processes are carried out in reactors providing greater surface to volume ratios than the presently used DME reactors. Certain embodiments of the processes are carried out in systems comprising multiple microchannel reactors.
摘要翻译： 公开了从甲醇生产二甲醚（DME）并直接从合成气生产DME的方法，例如来自生物质的合成气。 还公开了用于DME生产的装置。 所公开的方法通常在比常规方法更低的接触时间和更低的压力的较高温度下起作用，以产生比常规方法更高的DME产率。 该方法的某些实施方案在提供比目前使用的DME反应器更大的表面与体积比的反应器中进行。 该方法的某些实施方案在包括多个微通道反应器的系统中进行。
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10.发明授权Compact integrated combustion reactors, systems and methods of conducting integrated combustion reactions 有权紧凑的一体化燃烧反应器，进行综合燃烧反应的系统和方法公开(公告)号：US08696771B2
公开(公告)日：2014-04-15
申请号：US11611461
申请日：2006-12-15
CPC分类号： B01J19/249 , B01J19/0093 , B01J2219/00783 , B01J2219/00835 , B01J2219/00873 , B01J2219/2453 , B01J2219/2458 , B01J2219/2465 , B01J2219/2466 , B01J2219/2479 , C01B3/323 , C01B3/384 , C01B3/586 , C01B2203/0233 , C01B2203/0445 , C01B2203/047 , C01B2203/0811 , C01B2203/0822 , C01B2203/1064 , C01B2203/1076 , C01B2203/1223 , C01B2203/82 , Y02P20/128 , Y02P20/129
摘要： A compact integrated combustion reactor is described. In a preferred embodiment, the combustion catalyst is disposed in a staggered configuration such that the hot spot in an adjacent endothermic reaction chamber is substantially less than would occur with a conventional, unstaggered configuration. The integrated reactor may also include a methanation chamber for methanation of a reformate product. Systems containing reactant and product streams, and methods of conducting integrated combustion reactions are also described. A staggered catalyst conformation can be used more broadly for thermal chemical reactions requiring heat transfer in a layered device.
摘要翻译： 描述了紧凑的集成燃烧反应器。 在一个优选实施方案中，燃烧催化剂以交错构型设置，使得相邻吸热反应室中的热点基本上小于以常规的，未排列的构型发生的热点。 整合的反应器还可以包括用于重整产物的甲烷化的甲烷化室。 还描述了含有反应物和产物流的系统，以及进行集成燃烧反应的方法。 交错的催化剂构型可以更广泛地用于需要在分层器件中传热的热化学反应。
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