An organic semiconductor compound and a method for manufacturing the same are provided. The method for manufacturing the organic semiconductor compound includes stirring a solated organic semiconductor and a solated organometallic precursor to manufacture the organic semiconductor compound. Herein, the manufacturing the organic semiconductor compound includes: forming a three-dimensional organic semiconductor compound by allowing the solated organic semiconductor to orthogonally penetrate gaps in a lattice structure of a gelated organometallic precursor formed by stirring the solated organometallic precursor.