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公开(公告)号：US10087135B2
公开(公告)日：2018-10-02
申请号：US15743904
申请日：2015-12-08
发明人： Hongchao Liu , Wenliang Zhu , Youming Ni , Yong Liu , Zhongmin Liu , Linying Wang , Peng Tian
摘要： The present invention provides a method for producing a light fatty acid alkyl ester with the formula of R1—COO—R2, and the method comprises a step in which a alkyl ether with formula of R1—O—R2 and a raw gas containing carbon monoxide go through a reactor loaded with a catalyst for carrying out a carbonylation reaction; wherein the catalyst contains an acidic EMT zeolite molecular sieve; wherein R1 and R2 are independently selected from C1-C4 alkyl groups. The present invention has provided a new method for producing light fatty acid alkyl ester. In the method of the present invention, the carbonylation is carried out in the presence of the catalyst containing the acidic EMT zeolite molecular sieve, and the reaction activity is high, and the stability has been significantly improved, meeting the requirement of industrial production.
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公开(公告)号：US10822244B2
公开(公告)日：2020-11-03
申请号：US16321118
申请日：2016-08-02
发明人： Pengfei Wu , Miao Yang , Peng Tian , Zhongmin Liu , Linying Wang , Lin Liu
摘要： A method for synthesizing a nano SAPO-34 molecular sieve, and an SAPO-34 molecular sieve catalyst and application thereof. A nano SAPO-34 molecular sieve is synthesized by adding a microporous templating agent and a templating agent having a functionalized organic silane to hydrothermal synthesis. The nano SAPO-34 molecular sieve is calcined to obtain a nano SAPO-34 molecular sieve catalyst. The catalyst can be used in a reaction for preparing low-carbon olefin from an oxygen-containing compound. The nano SAPO-34 molecular sieve obtained by this method has a pure CHA crystal phase. Moreover, the nano SAPO-34 molecular sieve catalyst obtained by this method has good catalytic performance in a MTO reaction, the service life of the catalyst is significantly prolonged, and the selectivity of the low-carbon olefin is improved.
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公开(公告)号：US10968109B2
公开(公告)日：2021-04-06
申请号：US16467818
申请日：2016-12-09
发明人： Linying Wang , Peng Tian , Zhongmin Liu , Hongyi Yang , Xuebin Zhao , Beibei Gao , Yuyan Qiao
摘要： A method for synthesizing a mordenite (MOR) molecular sieve with a modulatable location and distribution of B acid sites, and a product thereof and the use thereof. Provided is a method for synthesizing a mordenite MOR molecular sieve with acid sites located at an 8-membered ring “side pocket” in communication with a 12-membered ring pore channel in the presence or absence of an inorganic base. The method includes introducing an additional reagent and an optional fluorinating reagent which have different structures and charge densities into a synthetic gel, and the B acid sites of the obtained MOR zeolite are located at an 8-membered ring “side pocket” in communication with a 12-membered ring pore channel A catalyst product obtained exhibits an excellent performance in terms of adsorption and catalysis. The synthesis method has broad industrial application, particularly being applied to catalysts for the carbonylation reaction of dimethyl ether.
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公开(公告)号：US10287233B2
公开(公告)日：2019-05-14
申请号：US15743936
申请日：2015-12-08
发明人： Hongchao Liu , Wenliang Zhu , Yong Liu , Youming Ni , Zhongmin Liu , Linying Wang , Peng Tian
IPC分类号： B01J29/70 , B01J29/74 , B01J29/76 , C07C67/37 , C07C69/14 , C07C29/147 , C07C51/377
摘要： The present invention provides a method for producing methyl acetate, and the method comprises a step in which dimethyl ether and a raw gas containing carbon monoxide and hydrogen go through a reactor loaded with a catalyst for carrying out a carbonylation reaction; wherein the catalyst contains an acidic EMT zeolite molecular sieve. The present invention has provided a new method for producing methyl acetate. In the method of the present invention, the carbonylation is carried out in the presence of the catalyst containing the acidic EMT zeolite molecular sieve, and the reaction activity is high, and the stability has been significantly improved, meeting the requirement of industrial production.
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