Multiphasic colorant nano-components (MPCs) having at least two phases and at least one colorant are provided. In certain aspects, the at least two phases are optically or visually distinct from one another. The MPCs can be used in various methods in various applications, such as visual, optical, and/or electronic displays, including in paints, inks, coatings, plastics, textiles, electronic display devices, pixels, or electronic paper. The MPCs are formed by methods of electrified jetting of polymers.