A display may have an array of pixels. Each pixel may have a light-emitting diode such as an organic light-emitting diode or may be formed from other pixel structures such as liquid crystal display pixel structures. The pixels may emit light such as red, green, and blue light. An angle-of-view adjustment layer may overlap the array of pixels. During operation, light from the pixels passes through the angle-of-view adjustment layer to a user. The viewing angle for the user is enhanced as the angular spread of the emitted light from the pixels is enhanced by the angle-of-view adjustment layer. The angle-of-view adjustment layer may be formed from holographic structures recorded by applying laser beams to a photosensitive layer or may be formed from a metasurface that is created by patterning nanostructures on the display using printing, photolithography, or other patterning techniques.