An anode of a lithium battery includes a supporting member and a carbon nanotube film disposed on a surface of the support member. The carbon nanotube film includes at least two overlapped and intercrossed layers of carbon nanotubes. Each layer includes a plurality of successive carbon nanotube bundles aligned in the same direction. A method for fabricating the anode of the lithium battery includes the steps of: (a) providing an array of carbon nanotubes; (b) pulling out, by using a tool, at least two carbon nanotube films from the array of carbon nanotubes; and (c) providing a supporting member and disposing the carbon nanotube films to the supporting member along different directions and overlapping with each other to achieving the anode of lithium battery.