This present invention is related to a method of collecting high-level radioactive contaminated uranium powder underwater. It utilizes a long rod fixed to the pipe of the sewage pump at bottom, and takes another end of the sewage pump to connect to the sediment bag to collect uranium powder which is dispersed and contaminates the pond. Inhaling the pond water contains uranium powder into the sediment bag by sewage pump that is joined to a collecting can under it and waiting for precipitation of the powder. When the uranium powder in the sediment bag is completely precipitated into the collecting can, operator can utilize submersible pump to drain the pond water from the sediment bag. Operator may hold the cable wire of the uranium powder collecting can manually to move it to the collecting shelf and repeat the process several times until the high-level radioactive uranium powder in the contaminated pond are all collected on the uranium powder collecting shelf.