The invention relates to a portable device for remotely measuring atmospheric pollution components day and night on the basis of a natural celestial body light source, which comprises a two-dimensional rotating platform system with a celestial body tracking function, a telescope system, a spectrometer and a computer. Received directly irradiated sunlight, moonlight, starlight and scattered sunlight are transmitted to the spectrometer by the telescope system through an optical fiber; spectral information acquired by the spectrometer is transmitted to the computer through AD (analog-to-digital) conversion; and the inversion is carried out by utilizing a related algorithm through the computer so as to obtain a vertical column concentration and vertical column distribution information of atmospheric trace gas. After the portable device for remotely measuring the atmospheric pollution components day and night is adopted, the day and night monitoring on the atmospheric conventional pollutant gas can be realized; and under the condition that any artificial light source is not required, a telescope is driven by a rotating platform to track a celestial body or carry out directional scanning so as to complete measuring a pollutant gas absorption spectrum. Compared with other optical methods, the portable device for remotely measuring the atmospheric pollution components day and night has the advantages that the portable device has simple system structure, is simple to assemble and disassemble and is convenient to carry; the day and night continuous measurement can be realized; and the vertical column concentration and the vertical column distribution information of the trace gas are obtained.